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O_2/CO_2气氛下燃煤过程中SO_2排放特性实验 被引量:15

Experiments of SO_2 emission characteristics during coal combustion under O_2/CO_2 atmosphere
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摘要 通过沉降炉对O2/CO2气氛和空气气氛下煤粉燃烧过程中SO2排放特性进行实验,结果表明,随燃料/氧化学当量比的增加,烟气中SO2浓度升高,单位煤生成SO2的量随燃料/氧化学当量比的增加而减少.在实验条件下,不加石灰石时,气氛和温度对SO2的生成无明显影响,SO2的生成量只与煤中含硫量以及煤的种类有关.当煤中加入石灰石后,O2/CO2气氛下SO2的排放量远小于空气气氛下,这主要是因为石灰石在O2/CO2气氛下取得的脱硫效率大大高于空气气氛下的脱硫效率. The experiments of SO2 emission characteristics during pulverized coal combustion were performed under O2/CO2 atmosphere and compared with air atmosphere. The results show that the SO2 concentration in flue gas increases and produced SO2 per gram decreases with increasing fuel/ oxygen equivalence ratio. The atmosphere and temperature have no influence on the quantity of released SO2 when no limestone is added. The quantity of released SO2 is only related to the content of sulfur and the kind of coal. With limestone added the released SO2 is much lower in O2/CO2 atmosphere than in air. This result is associated with the fact that the desulfurization efficiency of limestone is much higher in O2/CO2 atmosphere than in air.
出处 《东南大学学报(自然科学版)》 EI CAS CSCD 北大核心 2006年第4期546-550,共5页 Journal of Southeast University:Natural Science Edition
基金 国家重点基础研究专项经费基金资助项目(G1999022201-04)
关键词 O2/CO2气氛 煤粉燃烧 SO2排放 脱硫 石灰石 O2/CO2 atmosphere pulverized coal combustion SO2 emission desulfurization limestone
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参考文献11

  • 1Kiga T,Takano S,Kimura N.Characteristics of pulverized-coal combustion in the system of oxygen/recycled flue gas combustion[J].Energy Conversion and Management,1997,38(Sup):129-134.
  • 2Liu H,Okazaki K.Simultaneous easy CO2 recovery and drastic reduction of SOx and NOx in O2/CO2 coal combustion with heat recirculation[J].Fuel,2003,82(11):1427-1436.
  • 3Hayashi J-I,Hirama T,Okawa R,et al.Kinetic relationship between NO/N2O reduction and O2 consumption during flue-gas recycling coal combustion in a bubbling fluidized-bed[J].Fuel,2002,81(9):1179-1188.
  • 4Hosoda H,Hirama T,Azuma N,et al.NOx and N2O emission in bubbling fluidized-bed coal combustion with oxygen and recycled flue gas:macroscopic characteristics of their formation and reduction[J].Energy & Fuels,1998,12(1):102-108.
  • 5陈传敏,赵长遂,庞克亮,梁财.O_2/CO_2气氛下燃煤过程中NO_x排放特性实验研究[J].东南大学学报(自然科学版),2005,35(5):738-741. 被引量:22
  • 6Hu Y,Naito S,Kobayashi N,et al.CO2,NOx and SO2 emissions from the combustion of coal with high oxygen concentration gases[J].Fuel,2000,79(15):1925-1932.
  • 7Zaugg S D,Blackham A U,Hedman P O,et al.Sulfur pollutant formation during coal combustion[J].Fuel,1989,68(3):346-353.
  • 8Courtemanche B,Levendis Y A.A laboratory study on the NO,NO2,SO2,CO and CO2 emissions from the combustion of pulverized coal,municipal waste plastics and tires[J].Fuel,1998,77(3):183-196.
  • 9王宏,张礼知,邱建荣,郑楚光.高CO_2浓度下钙基吸收剂脱硫的实验研究[J].工程热物理学报,2001,22(3):374-377. 被引量:10
  • 10Liu H,Katagiri S,Kaneko U,et al.Sulfation behavior of limestone under high CO2concentration in O2/CO2 coal combustion[J].Fuel,2000,79(8):945-953.

二级参考文献20

  • 1[1]A M wolsky, E J Danniels, S Jody, et al.Recovering CO2 from Large and Medium-size Stationary Combustors.Journal of the Air and Waster Management Association, 1991, 41(4): 449-454
  • 2[2]Borgwardt R H, Sintering of Nascent Calcium Oxide.Chem. Eng. Sci., 1989, 44(1): 53-60
  • 3[1]Goldthorpe SH, Cross PJI, Davison JE, System studies on CO2 abatement from power plants[J]. Energy Convers Mgmt. ,1992,33(5-8): 459-466.
  • 4[2]Nakayama S, Noguchi Y. Pulverized coal combustion in O2/CO2 mixtures on a power plant for CO2 ecovery[J]. Energy Corverts. Mgnt.,1992,33(5-8): 379-386.
  • 5[3]Hu Y, Naito S, Kobayashi N, et al. CO2, NOx and SO2emission from the combustion of coal with high oxygen concentrationg ashes[J]. Fuel.2000,79: 1925-1932.
  • 6[4]Yamadea T, Kiga T, Okaua M, Characteristics of pulverized-coal combustion in CO2 ecovery power plant applied O2/CO2 [J]. JSME Entemational Journal, 1998, 41: 1017-1022.
  • 7[8]陈勤妹,黄瀛华,任德庆,等.应用TG-DTA-T-DTG和EGD-GC评价煤粉的燃烧特[J].华东理工大学学报,1997,23(6):286-291.Chen Qinmei,Huang Yinghua, Ren Deqing, et al. Evaluation of the combustion characteristic of pulverized coal by using TG-DTA-T-DTG and EGD-GC[J]. Journal of East China University of Science and Technology, 1997,23(6): 286-291.
  • 8[10]陈镜泓,立传儒.热分析方法及应用[M]北京:科学出版社,1985,124-127.
  • 9[11]任有中,钱剑青,房殿奇,等.180t/h煤粉炉内脱硫试验[J].锅炉技术,2002,33(4):29-32.Ren Youzhong,Qian Jianqing,Fang Dianqi et al. Desulfurization tests of 180t/h pulverized coal fired boiler by injecting desulphrizer[J]. Boiler Technology, 2002,33(4): 29-32.
  • 10[13]Fan L-S, Jiang P, Agnihotri R, Dispertion and ultra-fast reaction of calcium-based sorbent powders for SO2 and air toxics removal in coal combustion[J]. Chem. Eng. Sci, 1999,54: 5585-5597.

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