期刊文献+

N、Ce共掺杂TiO_2的制备及其光催化活性 被引量:1

Preparation and Photocatalytic Activity of Cerium and Nitrogen-codoped TiO_2
在线阅读 下载PDF
导出
摘要 采用溶胶-凝胶法制备沸石负载N、Ce共掺杂的二氧化钛光催化剂,以亚甲基蓝溶液为目标降解物研究该催化剂的光催化性能,并讨论催化剂浓度、pH值以及焙烧温度等对样品光催化性能的影响.结果表明:催化剂的焙烧温度为300℃时催化剂的催化活性最高,在反应体系中,催化剂浓度为60 g/L,pH=7时样品的光催化效率最佳,共掺杂的样品可见光活性高于单掺杂的样品.可见光辐射共掺杂的样品3 h,亚甲基蓝的去除率可以达65%. N and Ce co-doped TiO2 supported on artificial-zeolite (AZ) was prepared by sol-gel method. The photocatalytic activity was evaluated by degradation of methylene blue. The effects of amount of catalyst, the pH value and heating temperature on photocatalytic activity of the samples were discussed. The results indicated that the photocatalytic activity of co-doped photocatalyst was better than the single-doped photocatalyst. When the catalyst concentration was 60 g/L, the pH value was 7; the calcining temperature was 300 ℃, the photocatalytic activityt was best and degradation rate bereached 65% in 3 hours.
出处 《湖南城市学院学报(自然科学版)》 CAS 2012年第3期60-63,共4页 Journal of Hunan City University:Natural Science
基金 湖南省科技厅科研基金资助项目(2011FJ3174 2011GK3109)
关键词 光催化 沸石 TIO2 亚甲基蓝 photocatalytic zeolite TiO2 methylene blue
  • 相关文献

参考文献12

  • 1Vougioukalakis G. Stergiopoulos T, Kantonis G, et al. Terpyridine- and 2,6-dipyrazinylpyridme-coordinated ruthenium(II) complexes synthesis, characterization and application in TiO2-bascd dye-sansitized solar cells[J]. Journal of Photochemistry and Photobiology A: Chemistry, 2010: 214(1): 22-32.
  • 2MPimentel, N Oturan, M Dezotti, et al. Phenol degradation byadvanced elect-rochemical oxidation process electro-fenton usinga carbon felt cathode[J]. Applied Catalysis B: Environmental,2008,83(1-2): 140-149.
  • 3ShiJ W, Zheng J T, Hu Y,et al. Influnce of Fe3+ and Ho3+co-doping on the photocatalytic activity of TiC>2[J]. Mater ChemPhys, 2007, 106(2-3): 247-249.
  • 4GuD E,Yang B C, Hu Y D. V and N co-doped nanocrystalanatase TiO: photocatalysts with enhanced photocatalytic activityunder visible light irradiation[J]. Catalysis Communications, 2008,9(6): 1472-1476.
  • 5章晓彤,周国伟,白光伟.氮铈共掺杂介孔TiO_2的制备及在造纸废水处理中的应用[J].中国造纸,2010,29(2):28-31. 被引量:6
  • 6FujishimaA, Honda K. Electrochemical photolysis of water at asemiconduction electode[J]. Nature, 1972,238(5358): 37-38.
  • 7李英勃.负载型纳米Ti02光催化剂的制备及其在难降解有机废水处理中的应用研究[D].西安:西北大学,2001.
  • 8江海军,张瑾,奚丽荷,朱忠其,柳清菊.TiO_2半导体光催化剂在污水处理中的研究进展[J].材料导报,2007,21(F05):54-57. 被引量:13
  • 9吴建锋,叶韦韦,徐晓虹,饶正刚,成昊,葛海鹏.Eu^3+掺杂纳米TiO2光催化降解亚甲基蓝的研究[J].武汉理工大学学报,2011,33(1):14-17. 被引量:10
  • 10鲍长利,周波,刘淑霞,蒋引姗,方送生.沸石负载TiO_2的制备及其对农药敌敌畏的光降解性能[J].应用化学,2003,20(12):1222-1224. 被引量:9

二级参考文献66

共引文献74

同被引文献2

引证文献1

二级引证文献5

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部