We simultaneously investigate variations of a low order harmonic and photoelectron emission with an incident laser intensity by solving the time-dependent Schr6dinger equation in a momentum space. It can be found that...We simultaneously investigate variations of a low order harmonic and photoelectron emission with an incident laser intensity by solving the time-dependent Schr6dinger equation in a momentum space. It can be found that, the intensity of low order harmonic and photoelectron are gradually enhanced with the increase of the laser intensity, when the laser frequency is not in resonance with the transition frequency between the laser-induced high excited states and the ground state. If the resonance occurs, the intensity of the lower order harmonic is reduced and the interference can be observed in the lower order photoelectron spectra.展开更多
Using the time-dependent pseudo-spectral scheme, we solve the time-dependent Schrodinger equation of a hydrogen- like atom in a strong laser field in momentum space. The intensity-resolved photoelectron energy spectru...Using the time-dependent pseudo-spectral scheme, we solve the time-dependent Schrodinger equation of a hydrogen- like atom in a strong laser field in momentum space. The intensity-resolved photoelectron energy spectrum in abovethreshold ionization is obtained and further analyzed. We find that with the increase of the laser intensity, the abovethreshold ionization emission spectrum exhibits periodic resonance structure. By analyzing the population of atomic bound states, we find that it is the multi-photon excitation of bound state that leads to the occurrence of this phenomenon, which is in fairly good agreement with the experimental results.展开更多
We systematically investigate the influence of atomic potentials on the above-threshold ionization （ATI） spectra in one-dimensional （1D） cases and compare them with the three-dimensional （3D） case by numerically...We systematically investigate the influence of atomic potentials on the above-threshold ionization （ATI） spectra in one-dimensional （1D） cases and compare them with the three-dimensional （3D） case by numerically solving the time-dependent Schrrdinger equation. It is found that the direct ionization plateau and the rescattering plateau of the ATI spectrum in the 3D case can be well reproduced by the 1D ATI spectra calculated from the supersolid-core potential and the soft-core potential, respectively. By analyzing the factors that affect the yield of the ATI spectrum, we propose a modified-potential with which we can reproduce the overall 3D ATI spectrum. In addition, the influence of the incident laser intensities and frequencies on the ATI spectra calculated from the proposed modified potential is studied.展开更多
High-order harmonic generation(HHG)from an atom illuminated by a sinusoidally phase-modulated pulse is investigated by solving the time-dependent Schrödinger equation.The spectral shift that occurs in atomic HHG ...High-order harmonic generation(HHG)from an atom illuminated by a sinusoidally phase-modulated pulse is investigated by solving the time-dependent Schrödinger equation.The spectral shift that occurs in atomic HHG can be achieved easily using our laser pulse.It is shown that the photon energy of the generated harmonics is controllable within the range of 1 eV.The shift of the frequency peak position is rooted in the asymmetry of the rising and falling parts of the laser pulse.We also show that by varying the phase parameters in the frequency domain of the laser one can adjust and control the shift in atomic harmonic spectra.展开更多
We theoretically investigate the photoelectron emission from an atom irradiated by an amplitude modulated sinusoidally phase-modulated pulse through solving the time-dependent Schr¨odinger equation in the momentu...We theoretically investigate the photoelectron emission from an atom irradiated by an amplitude modulated sinusoidally phase-modulated pulse through solving the time-dependent Schr¨odinger equation in the momentum space. By controlling the phase amplitude of the pulse in the frequency domain, it can be found that the photoelectron spectra appear as explicit interference phenomena, which originated from the interference between the directly ionized electron and the ionization of the pre-excited atom from different subpulses.展开更多
We demonstrate that the interference minima in the linear molecular harmonic spectra can be accurately predicted by a modified two-center model. Based on systematically investigating the interference minima in the lin...We demonstrate that the interference minima in the linear molecular harmonic spectra can be accurately predicted by a modified two-center model. Based on systematically investigating the interference minima in the linear molecular harmonic spectra by the strong-field approximation （SFA）, it is found that the locations of the harmonic minima are related not only to the nuclear distance between the two main atoms contributing to the harmonic generation, but also to the symmetry of the molecular orbital. Therefore, we modify the initial phase difference between the double wave sources in the two-center model, and predict the harmonic minimum positions consistent with those simulated by SFA.展开更多
The duration of a bound electron tunneling through the barrier formed by atomic potential and electrostatic field is calculated by the Bohmian trajectories scheme. The time of the tunneling ionization decreases with t...The duration of a bound electron tunneling through the barrier formed by atomic potential and electrostatic field is calculated by the Bohmian trajectories scheme. The time of the tunneling ionization decreases with the increase of the amplitude of the electrostatic field. By using the information about the position, velocity and force of the Bohmian trajectories, the dynamical process of tunneling through the barrier is investigated.展开更多
We demonstrate theoretically that the high-order harmonic of an atom can be generated by a circularly polarized laser pulse.The harmonic spectrum shows a clear cutoff with an energy Ip ＋ 2Up.In particular,the high-or...We demonstrate theoretically that the high-order harmonic of an atom can be generated by a circularly polarized laser pulse.The harmonic spectrum shows a clear cutoff with an energy Ip ＋ 2Up.In particular,the high-order harmonic generation comes from the multiple recombination of the ionized electron with non-zero initial velocity.These results are verified by the classical model theory and the time-frequency analysis of a harmonic spectrum.展开更多
We theoretically investigate high-order harmonic generation from H ＋ 2 in an infrared laser field.Our numerical simulations show that a highly efficient plateau structure exists in the molecular harmonic spectrum.Und...We theoretically investigate high-order harmonic generation from H ＋ 2 in an infrared laser field.Our numerical simulations show that a highly efficient plateau structure exists in the molecular harmonic spectrum.Under the action of the infrared laser pulse,the bound electronic wave packet in a potential well has enough time to tunnel through the effective potential barrier,which is formed by the molecular potential and the infrared laser field,and then recombine with the neighboring nucleus emitting a harmonic photon.During the entire dynamic process,because the wave packet is mainly located in the effective potential,the diffusion effect is of no significance,and thus a highly efficient harmonic plateau can be achieved.Specifically,the cut-off frequency of the plateau is linearly scaled with the peak amplitude of the infrared laser electric field,which may open another route to examine the internuclear distance of the molecule.Furthermore,one may detect the molecular bond lengths using the harmonic plateau.展开更多
Using Bohmlan trajectory （151） method, we investigate the dynamic interference in nlgn-orcter narmonlc generauon from diatomic molecular ions. It is demonstrated that the main characteristics of the molecular harmon...Using Bohmlan trajectory （151） method, we investigate the dynamic interference in nlgn-orcter narmonlc generauon from diatomic molecular ions. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well reproduced by only two BTs which are located at the two ions. This haiapens because these two localized trajectories can receive and store the whole collision information coming from all of the other re-collision trajectories. Therefore, the amplitudes and frequencies of these two trajectories represent the intensity and frequency distribution of the harmonic generation. Moreover, the interference between these two trajectories shows a dip in the harmonic spectrum, which reveals the molecular structure information.展开更多
基金Project supported by the National Key Research and Development Program of China(Grant No.2017YFA0403300)the National Natural Science Foundation of China(Grant Nos.11774129,11274141,11627807,11604119,and 11534004)the Jilin Provincial Research Foundation for Basic Research,China(Grant No.20170101153JC)
文摘We simultaneously investigate variations of a low order harmonic and photoelectron emission with an incident laser intensity by solving the time-dependent Schr6dinger equation in a momentum space. It can be found that, the intensity of low order harmonic and photoelectron are gradually enhanced with the increase of the laser intensity, when the laser frequency is not in resonance with the transition frequency between the laser-induced high excited states and the ground state. If the resonance occurs, the intensity of the lower order harmonic is reduced and the interference can be observed in the lower order photoelectron spectra.
基金Project supported by the National Basic Research Program of China(Grant No.2013CB922200)the National Natural Science Foundation of China(Grants Nos.11274141,11034003,11304116,11274001,and 11247024)the Jilin Provincial Research Foundation for Basic Research,China(Grant No.20140101168JC)
文摘Using the time-dependent pseudo-spectral scheme, we solve the time-dependent Schrodinger equation of a hydrogen- like atom in a strong laser field in momentum space. The intensity-resolved photoelectron energy spectrum in abovethreshold ionization is obtained and further analyzed. We find that with the increase of the laser intensity, the abovethreshold ionization emission spectrum exhibits periodic resonance structure. By analyzing the population of atomic bound states, we find that it is the multi-photon excitation of bound state that leads to the occurrence of this phenomenon, which is in fairly good agreement with the experimental results.
基金Project supported by the National Basic Research Program of China(Grant No.2013CB922200)the National Natural Science Foundation of China(Grant Nos.11274141,11034003,11304116,11274001,and 11247024)the Jilin Provincial Research Foundation for Basic Research,China(Grant No.20140101168JC)
文摘We systematically investigate the influence of atomic potentials on the above-threshold ionization （ATI） spectra in one-dimensional （1D） cases and compare them with the three-dimensional （3D） case by numerically solving the time-dependent Schrrdinger equation. It is found that the direct ionization plateau and the rescattering plateau of the ATI spectrum in the 3D case can be well reproduced by the 1D ATI spectra calculated from the supersolid-core potential and the soft-core potential, respectively. By analyzing the factors that affect the yield of the ATI spectrum, we propose a modified-potential with which we can reproduce the overall 3D ATI spectrum. In addition, the influence of the incident laser intensities and frequencies on the ATI spectra calculated from the proposed modified potential is studied.
基金supported by the National Natural Science Foundation of China(Grant Nos.11604119,11627807,11774129,11774131,11904120,11975012,and 91850114)the Outstanding Youth Project of Taizhou University(Grant No.2019JQ002)。
文摘High-order harmonic generation(HHG)from an atom illuminated by a sinusoidally phase-modulated pulse is investigated by solving the time-dependent Schrödinger equation.The spectral shift that occurs in atomic HHG can be achieved easily using our laser pulse.It is shown that the photon energy of the generated harmonics is controllable within the range of 1 eV.The shift of the frequency peak position is rooted in the asymmetry of the rising and falling parts of the laser pulse.We also show that by varying the phase parameters in the frequency domain of the laser one can adjust and control the shift in atomic harmonic spectra.
基金Project supported by the National Key Research and Development Program of China(Grant No.2017YFA0403300)the National Natural Science Foundation of China(Grants Nos.11774129,11274141,11627807,11604119,and 11534004)the Jilin Provincial Research Foundation for Basic Research,China(Grant No.20170101153JC)
文摘We theoretically investigate the photoelectron emission from an atom irradiated by an amplitude modulated sinusoidally phase-modulated pulse through solving the time-dependent Schr¨odinger equation in the momentum space. By controlling the phase amplitude of the pulse in the frequency domain, it can be found that the photoelectron spectra appear as explicit interference phenomena, which originated from the interference between the directly ionized electron and the ionization of the pre-excited atom from different subpulses.
基金Project supported by the National Basic Research Program of China(Grant No.2013CB922200)the National Natural Science Foundation of China(Grant Nos.11274001,11274141,11304116,11247024,and 11034003)the Jilin Provincial Research Foundation for Basic Research,China(Grant Nos.20130101012JC and 20140101168JC)
文摘We demonstrate that the interference minima in the linear molecular harmonic spectra can be accurately predicted by a modified two-center model. Based on systematically investigating the interference minima in the linear molecular harmonic spectra by the strong-field approximation （SFA）, it is found that the locations of the harmonic minima are related not only to the nuclear distance between the two main atoms contributing to the harmonic generation, but also to the symmetry of the molecular orbital. Therefore, we modify the initial phase difference between the double wave sources in the two-center model, and predict the harmonic minimum positions consistent with those simulated by SFA.
基金Supported by the National Basic Research Program of China under Grant No 2013CB922200the National Natural Science Foundation of China under Grant Nos 11274141,11304116,11274001 and 11247024the Jilin Provincial Research Foundation for Basic Research under Grant No 20140101168JC
文摘The duration of a bound electron tunneling through the barrier formed by atomic potential and electrostatic field is calculated by the Bohmian trajectories scheme. The time of the tunneling ionization decreases with the increase of the amplitude of the electrostatic field. By using the information about the position, velocity and force of the Bohmian trajectories, the dynamical process of tunneling through the barrier is investigated.
基金Project supported by the National Basic Research Program of China (Grant No. 2013CB922200)the National Natural Science Foundation of China (GrantNos. 11274141 and 11034003)the Natural Science Foundation of Zhejiang Province of China (Grant No. Y6110578)
文摘We demonstrate theoretically that the high-order harmonic of an atom can be generated by a circularly polarized laser pulse.The harmonic spectrum shows a clear cutoff with an energy Ip ＋ 2Up.In particular,the high-order harmonic generation comes from the multiple recombination of the ionized electron with non-zero initial velocity.These results are verified by the classical model theory and the time-frequency analysis of a harmonic spectrum.
基金Project supported by the National Basic Research Program of China (Grant No. 2013CB922200)the National Natural Science Foundation of China (Grant Nos. 11274141 and 11034003)the Natural Science Foundation of Zhejiang Province,China (Grant No. Y6110578)
文摘We theoretically investigate high-order harmonic generation from H ＋ 2 in an infrared laser field.Our numerical simulations show that a highly efficient plateau structure exists in the molecular harmonic spectrum.Under the action of the infrared laser pulse,the bound electronic wave packet in a potential well has enough time to tunnel through the effective potential barrier,which is formed by the molecular potential and the infrared laser field,and then recombine with the neighboring nucleus emitting a harmonic photon.During the entire dynamic process,because the wave packet is mainly located in the effective potential,the diffusion effect is of no significance,and thus a highly efficient harmonic plateau can be achieved.Specifically,the cut-off frequency of the plateau is linearly scaled with the peak amplitude of the infrared laser electric field,which may open another route to examine the internuclear distance of the molecule.Furthermore,one may detect the molecular bond lengths using the harmonic plateau.
基金Project supported by the National Basic Research Program of China(Grant No.2013CB922200)the National Natural Science Foundation of China(Grant Nos.11274141,11034003,11304116,61275128,11247024,and 11274001)the Research Foundation for Basic Research of Jilin Province,China(Grant No.20140101168JC)
文摘Using Bohmlan trajectory （151） method, we investigate the dynamic interference in nlgn-orcter narmonlc generauon from diatomic molecular ions. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well reproduced by only two BTs which are located at the two ions. This haiapens because these two localized trajectories can receive and store the whole collision information coming from all of the other re-collision trajectories. Therefore, the amplitudes and frequencies of these two trajectories represent the intensity and frequency distribution of the harmonic generation. Moreover, the interference between these two trajectories shows a dip in the harmonic spectrum, which reveals the molecular structure information.
